Journal of Advanced Materials in Engineering

Journal of Advanced Materials in Engineering

Synthesis, Microstructural Characterization, and Mechanical Properties of a Layered Hybrid Aluminum-Matrix Composite Containing SiC Reinforcements and Iron-Based Amorphous Particles

Document Type : Original Article

Authors
School of Engineering, Damghan University, Damghan, Iran
Abstract
Introduction and Objectives: One effective approach for enhancing the mechanical properties of metal matrix composites is the design of architected layered heterogeneous structures. Hence, the present study aimed to develop aluminum matrix hybrid composites reinforced with SiC ceramic particles and iron-based amorphous particles, featuring a heterogeneous layered architecture and to investigate their mechanical properties.
Materials and Methods: The heterogeneous structure comprised alternating layers of pure aluminum and composite material with varying thicknesses, fabricated via powder metallurgy using spark plasma sintering (SPS). The microstructural and phase characteristics of the composites were investigated using scanning electron microscopy (SEM), optical microscopy (OM), and X-ray diffraction (XRD). The relationship between microstructure and mechanical properties was subsequently analyzed.
Results: Microstructural analyses, including porosity evaluation and density measurements, demonstrated enhanced densification during sintering with increasing pure aluminum layer thickness. In addition, the distribution of reinforcement particles was improved by increasing the volume fraction of the pure aluminum layers relative to the composite layers. Phase analysis of all sintered samples confirmed the preservation of the amorphous nature of the iron-based reinforcement particles and revealed no evidence of interfacial reaction products at the reinforcement–matrix interfaces. Mechanical experiments showed a favorable combination of high strength and ductility, with a compressive strength of up to 191 MPa and a fracture strain of 20% in samples with a higher volume fraction of composite layers. Furthermore, increased ductility was observed with a higher volume fraction of pure aluminum layers.
Conclusion: The introduction of a layered heterogeneous architecture in the hybrid composite, through modification of consolidation behavior and reinforcement particle distribution, resulted in superior mechanical properties compared to those of the homogeneous composite.
Keywords
Subjects

  1. Rezaei M, Albooyeh A, Chachei R, Malahi P. Effect of the spark plasma sintering temperature on the microstructure and mechanical properties of a ceramic/metallic glass reinforced hybrid composite. J Compos Mater. 2022;56(17):2779-88. https://doi.org/10.1177/00219983221078188
  2. Alem SAA, Sabzvand MH, Govahi P, Poormehrabi P, Hasanzadeh Azar M, Salehi Siouki S, et al. Advancing the next generation of high-performance metal matrix composites through metal particle reinforcement. Adv Compos Hyb Mater. 2025;8(1):3. https://doi.org/10.1007/s42114-024-01057-4
  3. Kumar A, SinghVP, Singh RC, Chaudhary R, Kumar D, Mourad AHI. A review of aluminum metal matrix composites: fabrication route, reinforcements, microstructural, mechanical, and corrosion properties. J Mater Sci. 2024.59(7):2644-2711. https://doi.org/10.1007/s10853-024-09398-7
  4. Abolkassem S , Elsayed A, Kariya S, Umeda J, Kondoh K. Influence of thermo-mechanical processing on microstructure and properties of bulk metallic glassy alloys-reinforced Al matrix composites prepared by powder metallurgy. J Mater Res Technol. 2023;7:8197-8208. https://doi.org/10.1016/j.jmrt.2023.11.225
  5. Zhai JT, Gao WJ, Dong HK, Hu Y-C, Zhang T, Zhu XG, et al. Novel metal matrix composites reinforced with Zr-based metallic glass lattices. Appl Mater Today 2022;29:101649. https://doi.org/10.1016/j.apmt.2022.101649
  6. Xie MS, Suryanarayana C, Zhao YL, Zhang WW, Yang C, Zhang GQ, et al. Abnormal hot deformation behavior in a metallic-glass-reinforced Al-7075 composite. Mater Sci Eng A 2020;785:139212. https://doi.org/10.1016/j.msea.2020.139212
  7. Dittmann K, Trauth A, Weidenmann KA. Manufacturing and characterization of an interpenetrating metal matrix composite reinforced with a 3D-printed metallic glass lattice structure (Ni60Nb20Ta20). Compos Str. 2024;327:117697. https://doi.org/10.1016/j.compstruct.2023.117697
  8. Rezaei M, Shabestari S, Razavi S. Investigation on equal-channel angular pressing-induced grain refinement in an aluminum matrix composite reinforced with Al-Cu-Ti metallic glass particles. J Mater Eng Perform. 2019;28:3031-40. https://doi.org/10.1007/s11665-019-04059-2
  9. Nomoto K, Ceguerra AV, Gammer C, Li B, Bilal H, Hohenwarter A, et al. Medium-range order dictates local hardness in bulk metallic glasses. Mater Today 2021;44:48-57. https://doi.org/10.1016/j.mattod.2020.10.032
  10. Bignoli F, Lemarchand A, Kalácska S, Thiaudiere D, Djemia P, Faurie D, et al. Extending mechanical size effect range of thin film metallic glasses by nanoengineering their atomic and nanostructure. Acta Mater. 2025;121456. https://doi.org/10.1016/j.actamat.2025.121456
  11. Dittmann K, Gruhl R, Trauth A, Weidenmann KA. In-situ failure behavior and interfacial bonding of an interpenetrating metal matrix composite reinforced with lattice-like metallic glass (Ni60Nb20Ta20) preform. Compos Struct. 2024;337:118084. https://doi.org/10.1016/j.compstruct.2024.118084
  12. Ertugrul O, He T, Shahid RN, Scudino S. Effect of heat treatment on microstructure and mechanical properties of Al 2024 matrix composites reinforced with Ni60Nb40 metallic glass particles. J Alloys Compds. 2019;808:151732. https://doi.org/10.1016/j.jallcom.2019.151732
  13. Guan HD, Li CJ, Gao P, Prashanth KG, Tan J, Eckert J, et al. Aluminum matrix composites reinforced with metallic glass particles with core-shell structure. Mater Sci Eng A 2020;771:138630. https://doi.org/10.1016/j.msea.2019.138630
  14. Huang L, Tan W, Li S, Li Y. Effect of loading pressure on mechanical properties and interface characteristics of 7056 Al alloy particle reinforced Zr-Al-Ni-Cu bulk metallic glass matrix composite prepared by spark plasma sintering. J Alloys Compds. 2020;816:152605. https:doi.org/10.1016/j.jallcom.2019.152605
  15. Birsen D, Tütük İ, Acar S, Karabeyoğlu SS, Özer G, Güler KA. Microstructure and wear characteristics of hybrid reinforced (ex-situ SiC–in-situ Mg2Si) Al matrix composites produced by vacuum infiltration method. Mater Chem Phys. 2023;302:127743. https://doi.org/10.1016/j.matchemphys.2023.127743
  16. Chinababu M, Bhaskar Rao E, Sivaprasad K. Fabrication, microstructure, and mechanical properties of Al-based metal matrix-TiB2 -HEA hybrid composite. J Alloys Compds. 2023;947: 169700. https://doi.org/10.1016/j.jallcom.2023.
  17. Ezatpour H, Torabi PM. Effect of carbonaceous hybrid reinforcement and extrusion temperature on the microstructure and mechanical properties of AA7075 matrix hybrid composite prepared by semi-solid casting. J Sci Technol Compos. 2021;8(1):1339-1352.
  18. Sharifian B, Borhani GH, Mohammad Sharifi E. Synthesis of Al7075/TiB2-Al2O3 in-situ hybrid composite by stir casting method. J Adv Mater Eng. 2022;41(2):51-65. https://doi.org/10.47176/jame.41.2.08071
  19. Zadali Mohammad kotiyani M, Ranjbar KH. The effect of heat treatment on the microstructure and mechanical properties of Al/Al3Zr + Al3Ti in-situ hybrid composite fabricated by friction stir processing. J Adv Mater Eng. 2017;38(1):49-64. https://doi.org/10.29252/jame.38.1.49
  20. Rezaei MR, Nazemnezhad R, Farahmandrad S. Effects of the Si element on the microstructure and mechanical properties of an Al/FMG/SiC hybrid composite. Mater Chem Phys. 2023;309:128343. https://doi.org/10.1016/j.matchemphys.2023.128343
  21. Shen M, Hao Z, Song J, An M, Ying T, Xue X, et al. Architectural and component design of CNTs/Al hierarchical composite for enhanced mechanical/thermal J Mater Res Technol. 2024;30:120-33. https://doi.org/10.1016/j.jmrt.2024.03.062
  22. Liu K, Cui Q, Shi L, Yang J, Cai Y, Su Y, et al. Grain structure tailoring strategy for heterogeneous lamella SiCp/2024Al composites with exceptional strength-ductility synergy. Compos B Eng. 2024;280:111491. https://doi.org/10.1016/j.compositesb.2024.111491
  23. Sun L, Zhang M, Zhong L, Liu C, Dou Y, Liu Y, et al. Designing strong and ductile heterogeneous lamella-structured Mg alloy via diffusion bonding. Mater Sci Eng A 2024;900:146489. https://doi.org/10.1016/j.msea.2024.146489
  24. ASTM B311-93. Test method for density determination for powder metallurgy (p/m) materials containing less than two percent porosity. West Conshohocken: ASTM International; 2020. https://www.astm.org/b0311-22.html
  25. Williamson G, Hall W. X-ray line broadening from filed aluminium and wolfram. Acta metal. 1953;1(1): 22-31. https://doi.org/10.1016/0001-6160(53)90006-6
  26. Warren B. X-ray Diffraction: Courier Corporation. North Chelmsford MA, USA; 1969.
  27. Zhao Y, Liao X, Jin Z, Valiev R, Zhu YT. Microstructures and mechanical properties of ultrafine grained 7075 Al alloy processed by ECAP and their evolutions during annealing. Acta Mater. 2004; 52(15):4589-99. https://doi.org/10.1016/j.actamat.2004.06.017
  28. ASTM E9-09. Standard test methods of compression testing of metallic materials at room temperature, ASTM International; West Conshohocken: 2020. https://www.astm.org/e0009-19.html
  29. Li X, Wang Y, Wang L, Xu M, Yi J. High thermal stability of residual amorphous regions in metallic glasses. Mater Lett. 2023;340:134210. https://doi.org/10.1016/j.matlet.2023.134210
  30. Jiang R, Torresani E, Olevsky EA. A Review of microstructure evolution and performance improvements in emerging sintering processes under controlled energy input. J Mat Res Technol. 2025; 39:368-391. https://doi.org/10.1016/j.jmrt.2025.09.129
  31. Airoldi L, Brucculeri R, Baldini P, Morganti S, Grande MA, Gobber FS, et al. Coupling direct powder deposition with spark plasma sintering: a new approach towards rapid prototyping. Prog Add Manu. 2024;9(6):1953-1966. https://doi.org/10.1007/s40964-023-00552-2
  32. Zeng X, Liu W, Xu B, Shu G, Li Q. Microstructure and mechanical properties of Al–Sic nanocomposites synthesized by surface-modified aluminium powder. Metals 2018.4(8):253. https://doi.org/10.3390/met8040253
  33. Tang S, Shao S, Liu H, Jiang F, Fu D, Zhang H, et al. Microstructure and mechanical behaviors of 6061 Al matrix hybrid composites reinforced with SiC and stainless steel particles. Mater Sci Eng A 2021;804: 140732. https://doi.org/10.1016/j.msea.2021.140732
  34. Najarian AR, Emadi R, Hamzeh M. Fabrication of as-cast Al matrix composite reinforced by Al2O3/Al3Ni hybrid particles via in-situ reaction and evaluation of its mechanical properties. Mater Sci Eng B 2018; 31:57-65. https://doi.org/10.1016/j.mseb.2018.09.002
  35. Maity T, Prakash A, Roy D, Prashanth KG. In situ Al3BC/Al composite fabricated via solid-solid reaction: An investigation on microstructure and mechanical behavior. App Sci. 2025;15(9):5189. https://doi.org/10.3390/app15095189

 

 


Articles in Press, Accepted Manuscript
Available Online from 09 February 2026

تحت نظارت وف بومی